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This work investigates the synthesis and computational characterization of a copper-based metal–organic framework (Cu-BDC-2) obtained by ionothermal synthesis using an ionic liquid as a template. Experimental and theoretical approaches (DFT+U and GFN1-xTB) were employed to evaluate its structural properties and CO₂ interactions, highlighting the influence of the ionic liquid on framework formation, surface properties, and adsorption behavior.
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